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ASTM_D_5281_-_98_2013.pdf

1、Designation:D528198(Reapproved 2013)Standard Test Method forCollection and Analysis of Hexavalent Chromium in AmbientAtmospheres1This standard is issued under the fixed designation D5281;the number immediately following the designation indicates the year oforiginal adoption or,in the case of revisio

2、n,the year of last revision.A number in parentheses indicates the year of last reapproval.Asuperscript epsilon()indicates an editorial change since the last revision or reapproval.1.Scope1.1 This test method covers the collection and measurementof hexavalent chromium Cr(VI)in the ambient atmosphere.

3、1.2 This test method collects and stabilizes atmospherichexavalent chromium using an alkaline impinger buffer solu-tion in a wet impingement sampling technique.Lead chromatePbCrO4,generally considered poorly soluble in water,issoluble in the impinger solution up to 940 g/L as hexavalentchromium.1.3

4、This test method measures hexavalent chromium usingan ion chromatographic separation combined with a postseparation reaction with a colorimetric reagent and photometricdetection.1.4 This test method is applicable in the range from 0.2 to100 ng/m3of hexavalent chromium in the atmosphere assum-ing 20

5、m3of air sample.The range can be extended upwards byappropriate dilution.1.5 The values stated in SI units are to be regarded as thestandard.The inch-pound units given in parentheses are forinformation only.1.6 This standard does not purport to address all of thesafety concerns,if any,associated wit

6、h its use.It is theresponsibility of the user of this standard to establish appro-priate safety and health practices and determine the applica-bility of regulatory limitations prior to use.2.Referenced Documents2.1 ASTM Standards:2D1193 Specification for Reagent WaterD1356 Terminology Relating to Sa

7、mpling and Analysis ofAtmospheresD1357 Practice for Planning the Sampling of the AmbientAtmosphereD2914 Test Methods for Sulfur Dioxide Content of theAtmosphere(West-Gaeke Method)D3195 Practice for Rotameter CalibrationD3586 Test Method for Chromium in Workplace Atmo-spheres(Colorimetric Method)(Wit

8、hdrawn 1990)33.Terminology3.1 Definitions:3.1.1 For definitions of terms used in this test method,referto Terminology D1356.3.2 Definitions of Terms Specific to This Standard:3.2.1 eluentthe ionic mobile phase used to transport thesample through the ion exchange column.3.2.2 resolutionthe ability of

9、 a column to separate con-stituents under specified test conditions.4.Summary of Test Method4.1 Sample Collection:4.1.1 Air is drawn at a rate of 15 L/min over a continuous24-h period through three 500-mL glass impingers(in-line)filled with 0.02 N sodium bicarbonate NaHCO3“buffer”solution.A target a

10、ir volume of 20 m3is sampled.4.1.2 Impinger buffer solution has a pH of 8.2 and wasselected to prevent hexavalent chromium from being reducedto trivalent chromium Cr(III)in an acidic medium duringsampling(1)4.4.1.3 The impinger buffer solution from each impinger isanalyzed for hexavalent chromium.4.

11、2 Sample Analysis(1,2,3,4):4.2.1 A volume of filtered sample,typically 1 mL,isinjected into the eluent flow path and separated by anionexchange using an ammonium sulfate(NH4)2SO4 basedeluent.4.2.2 After separation,the sample is reacted with an acidicsolution of diphenylcarbohydrazide.Hexavalent chro

12、mium1This test method is under the jurisdiction of ASTM Committee D22 on AirQuality and is the direct responsibility of Subcommittee D22.03 on AmbientAtmospheres and Source Emissions.Current edition approved Nov.1,2013.Published November 2013.Originallyapproved in 1992.Last previous edition approved

13、 in 2005 as D5281-98(2005).DOI:10.1520/D5281-98R13.2For referenced ASTM standards,visit the ASTM website,www.astm.org,orcontact ASTM Customer Service at serviceastm.org.For Annual Book of ASTMStandards volume information,refer to the standards Document Summary page onthe ASTM website.3The last appro

14、ved version of this historical standard is referenced onwww.astm.org.4The boldface numbers in parentheses refer to a list of references at the end ofthe text.Copyright ASTM International,100 Barr Harbor Drive,PO Box C700,West Conshohocken,PA 19428-2959.United StatesNOTICE:This standard has either be

15、en superseded and replaced by a new version or withdrawn.Contact ASTM International(www.astm.org)for the latest information1reacts selectively with this reagent to form the characteristicviolet colored complex.4.2.3 The eluent stream passes through a photometric de-tector for detection of the chromi

16、um diphenylcarbohydrazidecomplex by visible absorbance at 520 nm.Absorbance isproportional to the hexavalent chromium concentration.5.Significance and Use5.1 Hexavalent chromium has been shown to be a humanrespiratory carcinogen in epidemiological studies when hu-mans are exposed to relatively high airborne concentrations.Such high exposures may also induce dermal sensitization tohexavalent chromium in humans(5).5.2 Ambient atmospheric concentrations of hexavalentchromium are well below detectio

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